RT Journal Article T1 The influence of mixing on the stratospheric age of air changes in the 21st century A1 Eichinger, Roland A1 Dietmüller, Simone A1 Garny, Hella A1 Sacha , Petr A1 Birner, Thomas A1 Bönisch, Harald A1 Pitari, Giovanni A1 Visioni, Daniele A1 Stenke, Andrea A1 Rozanov, Eugene A1 Revell, Laura A1 Plummer, David A. A1 Jöckel, Patrick A1 Oman, Luke A1 Deushi, Makoto A1 Kinnison, Douglas E. A1 Garcia, Rolando A1 Morgenstern, Olaf A1 Zeng, Guang A1 Stone, Kane Adam A1 Schofield, Robyn K1 2502 Climatología K1 2501 Ciencias de la Atmósfera AB Climate models consistently predict an acceleration of theBrewer–Dobson circulation (BDC) due to climate change in the 21st century.However, the strength of this acceleration varies considerably amongindividual models, which constitutes a notable source of uncertainty forfuture climate projections. To shed more light upon the magnitude of thisuncertainty and on its causes, we analyse the stratospheric mean age of air(AoA) of 10 climate projection simulations from the Chemistry-Climate ModelInitiative phase 1 (CCMI-I), covering the period between 1960 and 2100. Inagreement with previous multi-model studies, we find a large model spread inthe magnitude of the AoA trend over the simulation period. Differencesbetween future and past AoA are found to be predominantly due to differencesin mixing (reduced aging by mixing and recirculation) rather than differencesin residual mean transport. We furthermore analyse the mixing efficiency, ameasure of the relative strength of mixing for given residual mean transport,which was previously hypothesised to be a model constant. Here, the mixingefficiency is found to vary not only across models, but also over time in allmodels. Changes in mixing efficiency are shown to be closely related tochanges in AoA and quantified to roughly contribute 10 % to the long-termAoA decrease over the 21st century. Additionally, mixing efficiencyvariations are shown to considerably enhance model spread in AoA changes. Tounderstand these mixing efficiency variations, we also present a consistentdynamical framework based on diffusive closure, which highlights the role ofbasic state potential vorticity gradients in controlling mixing efficiencyand therefore aging by mixing. PB Atmospheric Chemistry and Physics SN 16807324 YR 2019 FD 2019-01-24 LK http://hdl.handle.net/11093/4057 UL http://hdl.handle.net/11093/4057 LA eng NO Atmospheric Chemistry and Physics, 19(2): 921-940 (2019) NO Helmholtz Association | Ref. VH-NG-1014 DS Investigo RD 08-oct-2024